Silica-Based and Borate-Based, Titania-Containing Bioactive Coatings Characterization: Critical Strain Energy Release Rate, Residual Stresses, Hardness, and Thermal Expansion
Identifieur interne : 000519 ( Main/Exploration ); précédent : 000518; suivant : 000520Silica-Based and Borate-Based, Titania-Containing Bioactive Coatings Characterization: Critical Strain Energy Release Rate, Residual Stresses, Hardness, and Thermal Expansion
Auteurs : Omar Rodriguez ; Ali Matinmanesh ; Sunjeev Phull ; Emil H. Schemitsch [Canada] ; Paul Zalzal [Canada] ; Owen M. Clarkin ; Marcello Papini ; Mark R. Towler [Malaisie]Source :
- Journal of Functional Biomaterials [ 2079-4983 ] ; 2016.
Abstract
Silica-based and borate-based glass series, with increasing amounts of TiO2 incorporated, are characterized in terms of their mechanical properties relevant to their use as metallic coating materials. It is observed that borate-based glasses exhibit CTE (Coefficient of Thermal Expansion) closer to the substrate’s (Ti6Al4V) CTE, translating into higher mode I critical strain energy release rates of glasses and compressive residual stresses and strains at the coating/substrate interface, outperforming the silica-based glasses counterparts. An increase in the content of TiO2 in the glasses results in an increase in the mode I critical strain energy release rate for both the bulk glass and for the coating/substrate system, proving that the addition of TiO2 to the glass structure enhances its toughness, while decreasing its bulk hardness. Borate-based glass BRT3, with 15 mol % TiO2 incorporated, exhibits superior properties overall compared to the other proposed glasses in this work, as well as 45S5 Bioglass® and Pyrex.
Url:
DOI: 10.3390/jfb7040032
PubMed: 27916951
PubMed Central: 5197991
Affiliations:
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">Silica-Based and Borate-Based, Titania-Containing Bioactive Coatings Characterization: Critical Strain Energy Release Rate, Residual Stresses, Hardness, and Thermal Expansion</title><author><name sortKey="Rodriguez, Omar" sort="Rodriguez, Omar" uniqKey="Rodriguez O" first="Omar" last="Rodriguez">Omar Rodriguez</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation></author><author><name sortKey="Matinmanesh, Ali" sort="Matinmanesh, Ali" uniqKey="Matinmanesh A" first="Ali" last="Matinmanesh">Ali Matinmanesh</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation></author><author><name sortKey="Phull, Sunjeev" sort="Phull, Sunjeev" uniqKey="Phull S" first="Sunjeev" last="Phull">Sunjeev Phull</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation></author><author><name sortKey="Schemitsch, Emil H" sort="Schemitsch, Emil H" uniqKey="Schemitsch E" first="Emil H." last="Schemitsch">Emil H. Schemitsch</name><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation><affiliation wicri:level="1"><nlm:aff id="af3-jfb-07-00032">Department of Surgery, University of Western Ontario, London, ON N6A 4V2, Canada</nlm:aff><country xml:lang="fr">Canada</country><wicri:regionArea>Department of Surgery, University of Western Ontario, London, ON N6A 4V2</wicri:regionArea><wicri:noRegion>ON N6A 4V2</wicri:noRegion></affiliation></author><author><name sortKey="Zalzal, Paul" sort="Zalzal, Paul" uniqKey="Zalzal P" first="Paul" last="Zalzal">Paul Zalzal</name><affiliation><nlm:aff id="af4-jfb-07-00032">Oakville Trafalgar Memorial Hospital, Oakville, ON L6J 3L7, Canada;<email>paulzalzal@gmail.com</email></nlm:aff></affiliation><affiliation wicri:level="4"><nlm:aff id="af5-jfb-07-00032">Faculty of Health Sciences, Department of Surgery, McMaster University, Hamilton, ON L8S 4L8, Canada</nlm:aff><country xml:lang="fr">Canada</country><wicri:regionArea>Faculty of Health Sciences, Department of Surgery, McMaster University, Hamilton, ON L8S 4L8</wicri:regionArea><orgName type="university">Université McMaster</orgName><placeName><settlement type="city">Hamilton (Ontario)</settlement><region type="state">Ontario</region></placeName></affiliation></author><author><name sortKey="Clarkin, Owen M" sort="Clarkin, Owen M" uniqKey="Clarkin O" first="Owen M." last="Clarkin">Owen M. Clarkin</name><affiliation><nlm:aff id="af6-jfb-07-00032">School of Mechanical and Manufacturing Engineering, Dublin City University, Dublin D09 W6Y4, Ireland;<email>owen.clarkin@dcu.ie</email></nlm:aff></affiliation></author><author><name sortKey="Papini, Marcello" sort="Papini, Marcello" uniqKey="Papini M" first="Marcello" last="Papini">Marcello Papini</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation></author><author><name sortKey="Towler, Mark R" sort="Towler, Mark R" uniqKey="Towler M" first="Mark R." last="Towler">Mark R. Towler</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation><affiliation wicri:level="1"><nlm:aff id="af7-jfb-07-00032">Department of Biomedical Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia</nlm:aff><country xml:lang="fr">Malaisie</country><wicri:regionArea>Department of Biomedical Engineering, University of Malaya, Kuala Lumpur 50603</wicri:regionArea><wicri:noRegion>Kuala Lumpur 50603</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PMC</idno><idno type="pmid">27916951</idno><idno type="pmc">5197991</idno><idno type="url">http://www.ncbi.nlm.nih.gov/pmc/articles/PMC5197991</idno><idno type="RBID">PMC:5197991</idno><idno type="doi">10.3390/jfb7040032</idno><date when="2016">2016</date><idno type="wicri:Area/Pmc/Corpus">003150</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Corpus" wicri:corpus="PMC">003150</idno><idno type="wicri:Area/Pmc/Curation">003150</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Curation">003150</idno><idno type="wicri:Area/Pmc/Checkpoint">000459</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Checkpoint">000459</idno><idno type="wicri:Area/Ncbi/Merge">006C61</idno><idno type="wicri:Area/Ncbi/Curation">006C61</idno><idno type="wicri:Area/Ncbi/Checkpoint">006C61</idno><idno type="wicri:Area/Main/Merge">000519</idno><idno type="wicri:Area/Main/Curation">000519</idno><idno type="wicri:Area/Main/Exploration">000519</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a" type="main">Silica-Based and Borate-Based, Titania-Containing Bioactive Coatings Characterization: Critical Strain Energy Release Rate, Residual Stresses, Hardness, and Thermal Expansion</title><author><name sortKey="Rodriguez, Omar" sort="Rodriguez, Omar" uniqKey="Rodriguez O" first="Omar" last="Rodriguez">Omar Rodriguez</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation></author><author><name sortKey="Matinmanesh, Ali" sort="Matinmanesh, Ali" uniqKey="Matinmanesh A" first="Ali" last="Matinmanesh">Ali Matinmanesh</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation></author><author><name sortKey="Phull, Sunjeev" sort="Phull, Sunjeev" uniqKey="Phull S" first="Sunjeev" last="Phull">Sunjeev Phull</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation></author><author><name sortKey="Schemitsch, Emil H" sort="Schemitsch, Emil H" uniqKey="Schemitsch E" first="Emil H." last="Schemitsch">Emil H. Schemitsch</name><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation><affiliation wicri:level="1"><nlm:aff id="af3-jfb-07-00032">Department of Surgery, University of Western Ontario, London, ON N6A 4V2, Canada</nlm:aff><country xml:lang="fr">Canada</country><wicri:regionArea>Department of Surgery, University of Western Ontario, London, ON N6A 4V2</wicri:regionArea><wicri:noRegion>ON N6A 4V2</wicri:noRegion></affiliation></author><author><name sortKey="Zalzal, Paul" sort="Zalzal, Paul" uniqKey="Zalzal P" first="Paul" last="Zalzal">Paul Zalzal</name><affiliation><nlm:aff id="af4-jfb-07-00032">Oakville Trafalgar Memorial Hospital, Oakville, ON L6J 3L7, Canada;<email>paulzalzal@gmail.com</email></nlm:aff></affiliation><affiliation wicri:level="4"><nlm:aff id="af5-jfb-07-00032">Faculty of Health Sciences, Department of Surgery, McMaster University, Hamilton, ON L8S 4L8, Canada</nlm:aff><country xml:lang="fr">Canada</country><wicri:regionArea>Faculty of Health Sciences, Department of Surgery, McMaster University, Hamilton, ON L8S 4L8</wicri:regionArea><orgName type="university">Université McMaster</orgName><placeName><settlement type="city">Hamilton (Ontario)</settlement><region type="state">Ontario</region></placeName></affiliation></author><author><name sortKey="Clarkin, Owen M" sort="Clarkin, Owen M" uniqKey="Clarkin O" first="Owen M." last="Clarkin">Owen M. Clarkin</name><affiliation><nlm:aff id="af6-jfb-07-00032">School of Mechanical and Manufacturing Engineering, Dublin City University, Dublin D09 W6Y4, Ireland;<email>owen.clarkin@dcu.ie</email></nlm:aff></affiliation></author><author><name sortKey="Papini, Marcello" sort="Papini, Marcello" uniqKey="Papini M" first="Marcello" last="Papini">Marcello Papini</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation></author><author><name sortKey="Towler, Mark R" sort="Towler, Mark R" uniqKey="Towler M" first="Mark R." last="Towler">Mark R. Towler</name><affiliation><nlm:aff id="af1-jfb-07-00032">Department of Mechanical & Industrial Engineering, Ryerson University, Toronto, ON M5B 2K3, Canada;<email>amatinma@ryerson.ca</email> (A.M.);<email>sunjeev.phull@ryerson.ca</email> (S.P.);<email>mpapini@ryerson.ca</email> (M.P.);<email>mtowler@ryerson.ca</email> (M.R.T.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-jfb-07-00032">St. Michael’s Hospital, Toronto, ON M5B 1W8, Canada;<email>SchemitschE@smh.ca</email></nlm:aff></affiliation><affiliation wicri:level="1"><nlm:aff id="af7-jfb-07-00032">Department of Biomedical Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia</nlm:aff><country xml:lang="fr">Malaisie</country><wicri:regionArea>Department of Biomedical Engineering, University of Malaya, Kuala Lumpur 50603</wicri:regionArea><wicri:noRegion>Kuala Lumpur 50603</wicri:noRegion></affiliation></author></analytic><series><title level="j">Journal of Functional Biomaterials</title><idno type="eISSN">2079-4983</idno><imprint><date when="2016">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>Silica-based and borate-based glass series, with increasing amounts of TiO<sub>2</sub> incorporated, are characterized in terms of their mechanical properties relevant to their use as metallic coating materials. It is observed that borate-based glasses exhibit CTE (Coefficient of Thermal Expansion) closer to the substrate’s (Ti6Al4V) CTE, translating into higher mode I critical strain energy release rates of glasses and compressive residual stresses and strains at the coating/substrate interface, outperforming the silica-based glasses counterparts. An increase in the content of TiO<sub>2</sub> in the glasses results in an increase in the mode I critical strain energy release rate for both the bulk glass and for the coating/substrate system, proving that the addition of TiO<sub>2</sub> to the glass structure enhances its toughness, while decreasing its bulk hardness. Borate-based glass BRT3, with 15 mol % TiO<sub>2</sub> incorporated, exhibits superior properties overall compared to the other proposed glasses in this work, as well as 45S5 Bioglass<sup>®</sup> and Pyrex.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Webster, J B" uniqKey="Webster J">J.B. Webster</name></author><author><name sortKey="Chou, T" uniqKey="Chou T">T. Chou</name></author><author><name sortKey="Kenly, M" uniqKey="Kenly M">M. Kenly</name></author><author><name sortKey="English, M" uniqKey="English M">M. English</name></author><author><name sortKey="Roberts, T L" uniqKey="Roberts T">T.L. Roberts</name></author><author><name sortKey="Bloebaum, R D" uniqKey="Bloebaum R">R.D. Bloebaum</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Sullivan, J" uniqKey="Sullivan J">J. Sullivan</name></author><author><name sortKey="Uden, M" uniqKey="Uden M">M. 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Clarkin</name><name sortKey="Matinmanesh, Ali" sort="Matinmanesh, Ali" uniqKey="Matinmanesh A" first="Ali" last="Matinmanesh">Ali Matinmanesh</name><name sortKey="Papini, Marcello" sort="Papini, Marcello" uniqKey="Papini M" first="Marcello" last="Papini">Marcello Papini</name><name sortKey="Phull, Sunjeev" sort="Phull, Sunjeev" uniqKey="Phull S" first="Sunjeev" last="Phull">Sunjeev Phull</name><name sortKey="Rodriguez, Omar" sort="Rodriguez, Omar" uniqKey="Rodriguez O" first="Omar" last="Rodriguez">Omar Rodriguez</name></noCountry><country name="Canada"><noRegion><name sortKey="Schemitsch, Emil H" sort="Schemitsch, Emil H" uniqKey="Schemitsch E" first="Emil H." last="Schemitsch">Emil H. Schemitsch</name></noRegion><name sortKey="Zalzal, Paul" sort="Zalzal, Paul" uniqKey="Zalzal P" first="Paul" last="Zalzal">Paul Zalzal</name></country><country name="Malaisie"><noRegion><name sortKey="Towler, Mark R" sort="Towler, Mark R" uniqKey="Towler M" first="Mark R." last="Towler">Mark R. 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